But Acting Catalan President Artur Mas, who ran the Catalan government during years of national economic crisis that saw the independence movement swell, said the government of the wealthy northeastern region would stick to its plan.
"Legally, it is clear that the Catalan parliament`s resolution is now annulled," he said in an interview with Cadena Ser radio.
"But politically, it is not, because the will of the parliament cannot be annulled and the will of the parliament reflects the will and the ideas of a significant part of the Catalonian population."
The Constitutional Court ruled that the resolution was unconstitutional and said the Catalan assembly could not establish itself as an independent legal and political power above the constitution.
Mas said he wanted to hold another referendum on secession; an informal vote held last year produced a result of 81 percent in favor, although the turnout was only around 40 percent.
Parties favoring a split from Spain won a majority of seats in the Catalan parliament in September, but fell just short of half the vote.
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